Re: D&D again!
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PCGen comes bundled with the SRD, which is fine if you just want the basics (maybe best for newbies).
Effectively the 3 core books, plus Unearthed Arcana and Psionics Handbook.
If you want a more complete dataset, you'll have to find a homebrew one (or enter it all yourself).
One I'm aware of is by BahamutDragon. If you google that name, you should be able to find it.